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Aqueous-phase Hydrodechlorination of Trichloroethene over Pd-supported on Swellable Organically-modified Silica (SOMS)
Date
2016-11-16
Author
Çelik, Gökhan
Gunduz, Seval
Miller, Jeffrey T.
Tao, Franklin Feng
Edmiston, Paul L.
Ozkan, Umit S.
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https://hdl.handle.net/11511/74300
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Aqueous Phase Hydrodechlorination of Trichloroethylene Using Pd Supported on Swellable Organically Modified Silica (SOMS): Deactivation Due to Chloride and Sulfur Species
Ozkan, Umit S.; Ailawar, Saurabh A.; Hunoor, Anagha; Çelik, Gökhan; Gunduz, Seval; Miller, Jeffrey T.; Tao, Franklin Feng; Edmiston, Paul L. (2019-11-15)
Aqueous-Phase Hydrodechlorination of Trichloroethylene over Pd-Based Swellable Organically Modified Silica: Catalyst Deactivation Due to Sulfur Species
Çelik, Gökhan; Gunduz, Seval; Miller, Jeffrey T.; Edmiston, Paul L.; Ozkan, Umit S. (American Chemical Society (ACS), 2019-03-13)
One of the problems of catalytic water treatment systems is that sulfur-containing species present in contaminated water have a detrimental effect on the catalytic performance because of strong interactions of sulfur species with active metal sites. In order to address these problems, our research has focused on developing a poison-resistant catalytic system by using a novel material, namely, swellable organically modified silica (SOMS), as a catalyst scaffold. Our previous investigations demonstrated that ...
Aqueous Phase Hydrodechlorination of TCE with Pd Supported Swellable Organically Modified Silica(SOMS): Effect of Ethanol on Reaction Kinetics
Hunoor, A; Çelik, Gökhan; Özkan, Ümit S.; Miller, Jeffrey T; Edmiston, Paul L; Özkan, Ümit S (2020-12-01)
Aqueous-phase hydrodechlorination of trichloroethylene over Pd-based swellable organically-modified silica (SOMS): Catalyst deactivation due to chloride anions
Çelik, Gökhan; Gunduz, Seval; Miller, Jeffrey T.; Edmiston, Paul L.; Ozkan, Umit S. (Elsevier BV, 2018-12-30)
Swellable-organically modified silica (SOMS) has been demonstrated to be an efficient catalyst scaffold for catalytic treatment of water contaminated with trichloroethylene (TCE). In this study, deactivation characteristics of Pd-incorporated SOMS for aqueous-phase hydrodechlorination (HDC) of TCE were investigated. Pd/SOMS catalysts were exposed to highly-concentrated chloride solutions (up to 1 M NaCl or 0.01 M HCl) to examine the deactivation resistant behavior of Pd/SOMS. The commonly used HDC catalyst ...
Aqueous Self-Assembly of an Electroluminescent Double-Helical Metallopolymer
de Hatten, Xavier; Asil Alptekin, Demet; Friend, Richard H.; Nitschke, Jonathan R. (2012-11-21)
A new type of water-soluble copper-containing, polymer has been synthesized using the technique of subcomponent self-assembly. Copper(I)-directed imine bond formation between triethylene glycol functionalized 1,2-phenylenediamine and 2,9-diformylphenanthroline subcomponents resulted in the formation of a chain in which two conjugated helical ligand strands wrap around a linear array of metal ions. Characterization data from a variety of analytical methods are consistent with our formulation of this material...
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G. Çelik, S. Gunduz, J. T. Miller, F. F. Tao, P. L. Edmiston, and U. S. Ozkan, “Aqueous-phase Hydrodechlorination of Trichloroethene over Pd-supported on Swellable Organically-modified Silica (SOMS),” 2016, Accessed: 00, 2021. [Online]. Available: https://hdl.handle.net/11511/74300.